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UNSAFE RADWASTE
DISPOSAL AT WIPP
Dr. David Snow
PhD, Engineering Science University of California-Berkeley |
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Note:
In several places in his paper, Dr. Snow states that a near-surface
or above-ground, centralized, monitored retrievable storage facility,
possibly at WIPP, is now the only option to disposal at WIPP.
However, it is CARD's position that the WIPP waste should remain in
monitored retrievable storage at the generator sites while
research is pursued to find a truly safe method for final disposition
of this waste. The Department of Energy has stated that the WIPP
waste could stay safely at the generator sites for at least another
50 years. CARD believes that the risks from transporting 35,000
shipments of waste around the country to WIPP or another
centralized facility are great and outweigh the risks from properly
storing the waste where it is generated or currently stored.
The (Short Version) of this paper is also available in the Non-Technical Section.
Summary
At WIPP, radioactive waste is being disposed of permanently in
drums and boxes placed in rooms excavated in the Salado salt beds.
Like all other excavations below the water table, the repository will
saturate, and dissolved radioactivity can ultimately escape via
boreholes, shaft.s or fractures to the overlying Rustler evaporites.
The most evident aquifer in the Rustler, the Culebra dolomite, is
claimed by DOE to provide such slow transport that the Rustler can
be considered an adequate barrier to waste migration. But
performance assessment modeling, based on insufficient exploration
data, unsupportable deductions and faulty assumptions led to that
claim. This paper asserts that the Rustler formation overlying and
down-gradient of the WIPP repository will not provide the claimed
geologic containment because karst conduits are present that will
facilitate rapid, ephemeral flow. If disposal is not halted and timely
rectified, escaping radioactivity may reach Nash Draw within a
thousand years, contaminating the Pecos River and Rio Grande. Until
a suitable disposal site or method is engineered, a monitored
retrievable storage facility may offer the only alternative.
Introduction
In 1998, the Department of Energy (DOE) became certified to dispose
of transuranic (TRU) waste transported from military generation
sites around the country, placing it irretrievably in rooms excavated
in deep salt beds beneath the Waste Isolation Pilot Plant (WIPP),
Carlsbad, New Mexico, and is presently expanding the facility. The
urgency to eliminate surface stockpiles and to decontaminate bomb-
making plants and test facilities at Rocky Flats, Argonne, Arco,
Mound, Oak Ridge, Hanford, Savannah River, Nevada Test Site and the
Lawrence Livermore and Los Alamos Laboratories gave stimulus to
the conclusion that WIPP would provide safe, permanent isolation,
that excessive plutonium and other radionuclides will not be
conveyed in solution by groundwater moving from the repository
through covering rocks to the accessible environment (surface or 5
km distant) in less than the 10,000 years mandated by
40CFR191.
Deep geologic disposal has seemed to be the answer. Natural radioactivity in the biosphere results in mild carcinogenesis that humans accept, while uranium ore bodies that could not be tolerated are shielded by intervening thicknesses of rock. Low solubility of ore minerals, and dilution and slow transport as solutes in groundwater have protected us. But in the last half-century, mining and processing of uranium ore, fission, bomb manufacture, and waste reprocessing have concentrated uranium and transuranic elements at numerous accessible places. It is logical to reverse the destination of the radionuclides, such as plutonium and americium resulting from bomb making, by burying these wastes deep in the earth. But such geologic disposal methods have proven so difficult to validate that every nuclear nation remains burdened with dangerous stockpiles of spent fuel, unneeded bomb triggers and contaminated materials. WIPP is the first and only permitted disposal facility in the world for TRU wastes. But because adequate containment conditions were not proven at the WIPP site, the facility does not make the case for safe geologic disposal. A single monitored retrievable surface or near-surface facility may be the most prudent U.S. repository until a better technology develops. Various geologic media have been studied as potential hosts for
the permanent disposal of U.S. radwastes. Crystalline rocks,
including granite, basalt and metamorphics, though possessing low
permeabilities that assure slow transport rates, were disqualified
because all sites are water-saturated and connected to potable
water sources. Though pervasive but tight fractures are the typical
conduits for leakage, it has never been possible to prove the absence
of preferred pathways, such as fault zones, that would shorten
travel-times to streams or aquifers. Since 1957, rock salt has been
considered a favorable medium because of the perception of a nearly
impermeable, self-sealing nature. However, abandoned salt mines
near Lyons, Kansas were disqualified in 1972 because the overburden
rocks are perforated by many old drill holes. Salt domes of the Gulf
Coast region were considered but disqualified due to the probability
that fluids in a sealed cavern subject to creep closure would be
ejected, ultimately reaching overlying aquifers. WIPP is similar in
these regards. Bedded salt near Hereford, Texas failed as a candidate
by decree of an economy-minded Congress, together with the
candidate site in basalt at Hanford, Washington. That left. for active
investigation only a site in welded tuff at Yucca Mountain, Nevada
for civilian power-plant radwastes, and bedded salt at WIPP for
military radwastes. Though high permeability and deep drainage of
the fractured tuff at Yucca Mountain provides an unsaturated
environment, remaining uncertainties of future climate conditions,
faulting, volcanism and seismically-driven hydrothermal upwelling
(Hill, et. al. , 1995; Hill and Dublyansky, 1999) cast doubts on the
adequacy of waste isolation there.
The Hydrogeologic Setting of WIPP
The underground facility lies 2,150 ft. below the surface and is
ultimately to measure 4350 by 5050 ft. in dimensions, a significant
part of the Land Withdrawal Area (LWA, Figure 1), often referred to as the site. The geology
has been summarized by Powers, et. al., (1978) and Brinster
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Performance Assessment
Repository performance is judged according the radioactivity
accumulated over 10,000 years outside the accessible environment
boundary. Limits in Curies based on health effects at a surface body
of water are prescribed by the EPA in 40 CFR 191.13 for all
radionuclides in the expected inventory of materials disposed.
Performance Assessment (PA) is a modeling exercise of prodigious
complexity (Helton, et. al., 2000), designed to take into
consideration all physical properties of the wastes, the repository
and its geologic environs, including effects of climate and man-
made perturbations. It is a collection of models, each of which
embodies a time-dependent mathematical representation, a method
of numerical evaluation and a computer code. There is a model to
represent the two-phase inflow and outflow of brine and gas
between a sealed repository and anhydrite beds in the salt a few
feet above and below the repository horizon. There is a model to
calculate the hydrogen that will evolve from the reaction of brine
with disintegrating steel drums and cellulose in the waste. There is
a model to calculate the changing radionuclide inventory as it
decays, dissolves in the brine and is absorbed by engineered backfill
materials. There is a model to describe the groundwater flow in the
Culebra dolomite aquifer (assumed to be the sole conduit) above the
repository, and a model to calculate transport of each radionuclide
species through time and distance along Culebra pathways. PA
incorporates several different scenarios, such as no human
disturbance during the 10,000 years, or mining of potash in the
overlying McNutt Member of the Salado, or oil-well interceptions of
the repository and/or pressurized brine reservoirs in the underlying
Castile Formation, plus implications of borehole drilling, plugging
and blowout prevention. Because a single PA requires many man-
years of effort and millions of dollars worth of Cray CPU time, few
have been done. Scores of physical properties are factors in the
computations, many of which are ill-defined, so are best described
as distributions. The methods of Monte-Carlo sampling are used,
several hundred iterations providing a range of answers, each a
distribution function of the cumulative releases over the 10,000
years. The proportion of iterations that satisfy the EPA criteria
measures the probability of acceptable results. Any scientist has to
admire the elegance of the computation procedure even if his
expertise covers only a part, while the manager or politician reveres
that which is understandably baffling. But scrutiny reveals that
underlying the mathematical elegance and the comprehensive array
of data manipulated are numerous assumptions, many of which have
over-riding significance to the results. Some of the hydrogeological
assumptions violate the perceptions of qualified critics, such as
Anderson, 1978, Ferrall and Gibbons, 1980, Barrows, 1982, Snyder,
1985, Phillips, R. H., 1987, Snow, 1998 and Hill, 1999, and arguably
differ from actual conditions. Management has exerted its will to
succeed in the licensing process, influencing the scientific staff to
adopt models and select studies favorable to Doe's objectives,
biasing the results of PA. A critic must use Doe's own data and draw
inferences from his own observations to show where investigations
have gone astray. There are areas of geology, rock mechanics and
hydrology that deserve re-assessment in that light.
Contaminated Brine Discharge from the Repository
The starting point for all PA model realizations is the calculation of
brine inflows aft.er the repository is filled and sealed. As noted by
Brinster (1989, p. II-19), the Salado is not homogeneous salt, but
rather, . . . consists of salt rhythmically interbedded with
anhydrite, polyhalite, some glauberite, and some thin
mudstones. The salt was formerly believed to be so
impermeable that the rooms would remain dry, but the appearance of
small brine seeps soon aft.er opening the first research rooms
showed that DOE must contend with a wet waste environment.
Excepting direct recovery of solid waste carried to the surface along
with cuttings from inadvertent oil wells, all other scenarios entail
radionuclide transport via flowing groundwater. The project might
have been aborted if DOE had been more respectful of the historic
problems of water in salt and potash mining. At WIPP, brine that
accumulates will eventually saturate downdip openings, corrode
containers and packaging and dissolve radionuclides. Generated gas
will collect updip. The computed brine inflows depend on the
measured permeabilities of fractured anhydrite beds above and
below the repository horizon, but only the 3.0-ft. thick Marker Bed
#139, 9.5-ft. below the repository floor, Marker Beds A and B,
totaling 0.7 ft. thick and lying 4.3 ft. above the roof and the 0.6-ft.
Marker Bed #138, 39.2 ft. above the roof have been modeled as
inflow contributors. That limitation was due to the assumed extent
of the DRZ, the disturbed rock zone (fractured salt) expected to form
around the rooms as they close. The consequences of gas generation,
cavity pressurization and two-phase outflows of brine and gas
through those four anhydrite beds indicated (by PA) that the
undisturbed scenario poses no hazard of a significant breach or
accumulation beyond the accessible environment.
The fallacy of that conclusion stems from a misconception of the behavior of the Salado overburden. The 13-ft. high by 33-ft. wide rooms will be short-lived. Large open fractures appear in the ceilings of all rooms within months of mining. Several roof-falls and floor heaves have already occurred, so an extensive array of roof bolts has been installed to delay the failure of the remaining experimental rooms long enough to fill them with drums. These, and all future rooms will suffer collapse of major roof slabs bounded above by weak clay-bed partings. Such falls will crush the drums, and liberated waste will penetrate the fractures. DOE has assumed roof fractures extending upwards only to Marker Bed #138, but as creep subsidence incorporates whole panels and then the repository width, horizontal slip and openings will occur on successive higher clay seams, most bounding stiff anhydrites. Horizontal slickensides observed in Rustler clays at the Exhaust Shaft. (Holt and Powers, 1986) manifest the shear failure to be expected in Salado clay seams, a consequence of local subsidence. Inclined fractures laterally limiting roof slabs will interconnect the rooms and panels via the slip surfaces and fractured anhydrite beds situated farther above the repository, each of which will contribute to increasing inflows of brine. Experience at potash mines in similar salt sequences (notably at K-2 Mine in Saskatchewan) indicate that such roof behavior is typical. At the Canadian mines, the fractures sometimes breach the top of salt into an aquifer, causing inflows that flood the mine (Tofani, R., 1983, Van Sambeek, 1993). Aft.er shaft. leakage, such roof breaching is the next most common cause of flooding of salt and potash mines, all of which ultimately flood because they lie below the water table and have inhomogeneous, deforming roof-rocks. Such subsidence experience invalidates the assumed limited height of the disturbed rock zone around WIPP rooms and the continuous plastic creep and room closure envisioned by the designers. Fundamental to subsidence prediction at WIPP is that ultimately, inclined fractures, as shown by MacIntosh (1990) will bound a de-stressed region extending over entire panels of rooms. Because each anhydrite bed (numbering about 40 above the repository) has a thin, weak clay parting at each of its faces, the bedded, subsiding roof will be split into many independent beams, like a glu-lam beam that has come unglued. The deflections and accompanying inclined fractures will drain not just Marker Beds #138 and #139, plus A and B, but many more anhydrite beds above them, increasing the inflow rates accordingly. Some fractures extending up from the repository will not anneal, but because of movement and flow, will remain open for gas and brine leakage during the years of pressurization by closure and gas generation. Far-field pore pressures approaching lithostatic in salt not only drive the brine inflows along the anhydrites and clays, but also ensure that little subsequent outflow follows the bedding during pressurization. In PA, the Salado above anhydrite marker #138 up to the Rustler is assumed to be salt with very low permeability distributed uniformly around a median of 6.1 X 10-20 ft..2. Utilizing Darcy's Law (Helton, 1991, p. 83 and Table 4), flow upward across the 1300 ft. of salt (about 85%) and fractured anhydrite beds (about 15%) up to the Culebra dolomite aquifer was computed as though the interval is a continuous porous medium. What is significantly wrong with the model is that it assumes no fracture conduits reaching high above the panels. Rather, as pressures in the sealed repository rise, gasses will cause the subsidence fractures to propagate unstably to higher levels where smaller rock stresses prevail, facilitating subsequent brine leakage to the Culebra and other aquifers much sooner and at higher rates than the PA model predicts. Because of the non-conservative assumption that the Salado is structureless, and consequently because the rock mechanics model is unrealistic of long-term subsidence, the conclusion from PA calculations that the undisturbed scenario is innocuous has to be wrong. Histories and subsidence behavior of the analogous Salado interval above the McNutt horizon at nearby potash mines of Eddy County, NM could have been studied, reported and modeled, to derive more realistic WIPP- site subsidence predictions. Sandia rock mechanics wanted to do that at the Horizon (Amax) Mine (Crosser, 1998), but funding was denied them. It is common geotechnical experience that in a significant proportion of dams, tunnels, aqueducts or deep mines, if there are potential but unknown geologic defects or mechanical inhomogeneities, failure will occur by reason of unexpected hydrologic effects. Therefore, in sensitive and doubtful situations, especially conservative assumptions are appropriate. Instead, WIPP modeling employed idealistic assumptions of continuous media, when discontinuous (fracture) properties would have been appropriate. The conservative expectation is that subsidence fractures at WIPP will propagate first by gravity, then unstably upwards to the Rustler due to the gas pressure generated in the repository, followed by contaminated brines aft.er the gas has dissipated and rooms become saturated. Sealed shaft.s and boreholes nearby will probably retain their integrity unchallenged, because fractures will provide easier egress for fluids. There is currently a concentrated leakage occurring into the Construction and Salt Handling Shaft. from the top of Dewey Lake redbeds at 20 to 70 ft. in depth, thence into the repository, believed to arise from runoff at the parking lot. In European potash mining experience, such incipient karstic shaft. leakage has been found to be irreparable. The first drop of water signals the eventual flooding of the mine.
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